Estimated rate of cesium-137 emission from the Fukushima Daiichi nuclear plant, 10-24 March 2011. Modeling the first week of the Fukushima disaster reveals that huge bursts of radioisotopes poured from reactors and a spent-fuel storage pond. nature.com / Stohl, A. et al. Atmos. Chem. Phys. Discuss. 11, 28319-28394 (2011)

By Geoff Brumfiel, with additional reporting by David Cyranoski and Rina Nozawa
25 October 2011 The disaster at the Fukushima Daiichi nuclear plant in March released far more radiation than the Japanese government has claimed. So concludes a study1 that combines radioactivity data from across the globe to estimate the scale and fate of emissions from the shattered plant. The study also suggests that, contrary to government claims, pools used to store spent nuclear fuel played a significant part in the release of the long-lived environmental contaminant cesium-137, which could have been prevented by prompt action. The analysis has been posted online for open peer review by the journal Atmospheric Chemistry and Physics. Andreas Stohl, an atmospheric scientist with the Norwegian Institute for Air Research in Kjeller, who led the research, believes that the analysis is the most comprehensive effort yet to understand how much radiation was released from Fukushima Daiichi. “It’s a very valuable contribution,” says Lars-Erik De Geer, an atmospheric modeler with the Swedish Defense Research Agency in Stockholm, who was not involved with the study. The reconstruction relies on data from dozens of radiation monitoring stations in Japan and around the world. Many are part of a global network to watch for tests of nuclear weapons that is run by the Comprehensive Nuclear-Test-Ban Treaty Organization in Vienna. The scientists added data from independent stations in Canada, Japan and Europe, and then combined those with large European and American caches of global meteorological data. Stohl cautions that the resulting model is far from perfect. Measurements were scarce in the immediate aftermath of the Fukushima accident, and some monitoring posts were too contaminated by radioactivity to provide reliable data. More importantly, exactly what happened inside the reactors — a crucial part of understanding what they emitted — remains a mystery that may never be solved. “If you look at the estimates for Chernobyl, you still have a large uncertainty 25 years later,” says Stohl. Nevertheless, the study provides a sweeping view of the accident. “They really took a global view and used all the data available,” says De Geer. […] The latest report from the Japanese government, published in June, says that the plant released 1.5 × 1016  becquerels of cesium-137, an isotope with a 30-year half-life that is responsible for most of the long-term contamination from the plant2. A far larger amount of xenon-133, 1.1 × 1019 Bq, was released, according to official government estimates. The new study challenges those numbers. On the basis of its reconstructions, the team claims that the accident released around 1.7 × 1019 Bq of xenon-133, greater than the estimated total radioactive release of 1.4 × 1019  Bq from Chernobyl. The fact that three reactors exploded in the Fukushima accident accounts for the huge xenon tally, says De Geer. Xenon-133 does not pose serious health risks because it is not absorbed by the body or the environment. Cesium-137 fallout, however, is a much greater concern because it will linger in the environment for decades. The new model shows that Fukushima released 3.5 × 1016  Bq cesium-137, roughly twice the official government figure, and half the release from Chernobyl. The higher number is obviously worrying, says De Geer, although ongoing ground surveys are the only way to truly establish the public-health risk. […]

Fallout forensics hike radiation toll